Influence of tropospheric SO2emissions on particle formation and the stratospheric humidity


Contact
mrex [ at ] awi-potsdam.de

Abstract

Stratospheric water vapor plays an important role in the chemistry and radiation budget of the stratosphere. Throughout the last decades stratospheric water vapor levels have increased and several processes have been suggested to contribute to this trend. Here we present a mechanism that would link increasing anthropogenic SO2 emissions in southern and eastern Asia with an increase in stratospheric water. Trajectory studies and model simulations suggest that the SO2 increase results in the formation of more sulfuric acid aerosol particles in the upper tropical troposphere. As a consequence, more ice crystals of smaller size are formed in the tropical tropopause, which are lifted into the stratosphere more readily. Our model calculations suggest that such a mechanism could increase the amount of water that entered the stratosphere in the condensed phase by up to 0.5 ppmv from 1950-2000. Copyright 2005 by the American Geophysical Union.



Item Type
Article
Authors
Divisions
Programs
Publication Status
Published
Eprint ID
10923
DOI https://www.doi.org/10.1029/2004gl022159

Cite as
Notholt, J. , Luo, B. , Fueglistaler, S. , Weisenstein, D. , Rex, M. , Lawrence, M. , Bingemer, H. , Wohltmann, I. , Corti, T. , Warneke, T. , von Kuhlmann, R. and Peter, T. (2005): Influence of tropospheric SO2emissions on particle formation and the stratospheric humidity , Geophysical Research Letters, 32 (7), n/a-n/a . doi: https://www.doi.org/10.1029/2004gl022159


Share


Citation

Research Platforms
N/A

Campaigns
N/A


Actions
Edit Item Edit Item