Aerosol decadal trends – Part 2: In-situ aerosol particle number concentrations at GAW and ACTRIS stations


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Rolf.Weller [ at ] awi.de

Abstract

<jats:p>Abstract. We have analysed the trends of total aerosol particle number concentrations (N) measured at long-term measurement stations involved either in the Global Atmosphere Watch (GAW) and/or EU infrastructure project ACTRIS. The sites are located in Europe, North America, Antarctica, and on Pacific Ocean islands. The majority of the sites showed clear decreasing trends both in the full-length time series, and in the intra-site comparison period of 2001–2010, especially during the winter months. Several potential driving processes for the observed trends were studied, and even though there are some similarities between N trends and air temperature changes, the most likely cause of many northern hemisphere trends was found to be decreases in the anthropogenic emissions of primary particles, SO2 or some co-emitted species. We could not find a consistent agreement between the trends of N and particle optical properties in the few stations with long time series of all of these properties. The trends of N and the proxies for cloud condensation nuclei (CCN) were generally consistent in the few European stations where the measurements were available. This work provides a useful comparison analysis for modelling studies of trends in aerosol number concentrations. </jats:p>



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Eprint ID
30897
DOI https://www.doi.org/10.5194/acp-13-895-2013

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Asmi, A. , Collaud Coen, M. , Ogren, J. , Andrews, E. , Sheridan, P. , Jefferson, A. , Weingartner, E. , Baltensperger, U. , Bukowiecki, N. , Lihavainen, H. , Kivekäs, N. , Asmi, E. , Aalto, P. , Kulmala, M. , Wiedensohler, A. , Birmili, W. , Hamed, A. , O'Dowd, C. , G Jennings, S. , Weller, R. , Flentje, H. , Fjaeraa, A. , Fiebig, M. , Myhre, C. , Hallar, A. , Swietlicki, E. , Kristensson, A. and Laj, P. (2013): Aerosol decadal trends – Part 2: In-situ aerosol particle number concentrations at GAW and ACTRIS stations , Atmospheric Chemistry and Physics, 13 (2), pp. 895-916 . doi: https://www.doi.org/10.5194/acp-13-895-2013


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